Topology reveals the hidden rules of amorphous materials — Softness arises from hierarchical structures
For decades, the origins of “soft spots” in amorphous materials like glass remained a mystery. A new study shows that hierarchical atomic structures, uncovered through mathematical topology, are responsible for their mechanical behavior.
2025-09-25
(Press-News.org)
Osaka, Japan — Why do glass and other amorphous materials deform more easily in some regions than in others? A research team from The University of Osaka, the National Institute of Advanced Industrial Science and Technology (AIST), Okayama University, and the University of Tokyo has uncovered the answer. By applying a mathematical method known as persistent homology, the team demonstrated that these soft regions are governed by hidden hierarchical structures, where ordered and disordered atomic arrangements coexist.
Crystalline solids, such as salt or ice, have atoms neatly arranged in repeating patterns. Amorphous materials, including glass, rubber, and certain plastics, lack this long-range order. However, they are not completely random: they possess medium-range order (MRO), subtle atomic patterns that extend over a few nanometers.
MRO has long been suspected to play a critical role in determining the physical properties of amorphous materials, particularly their mechanical responses. Yet, because of the complexity of atomic networks, conventional analysis methods have been unable to clarify how MRO relates to regions that deform more easily than their surroundings. The structural origins of mechanical softness in amorphous solids have therefore remained elusive.
The research team applied persistent homology, a branch of topological data analysis that captures structural features across multiple scales. In amorphous silicon—a prototypical covalent amorphous material widely used in solar cells and electronic devices—they discovered hierarchical ring structures: smaller rings with irregular edge lengths are nested inside larger rings.
This coexistence of order and disorder means that softness emerges not from randomness alone, but from constraints imposed by medium-range order interwoven with local disorder. The study also revealed that these hierarchical structures strongly correlate with low-energy localized vibrations, a universal feature of glasses known as the “boson peak.”
“This work provides a new route to link the atomic structure of amorphous materials with their mechanical responses,” says Emi Minamitani of The University of Osaka, the lead author of the study. “We believe these insights will accelerate the design of durable glass and other advanced amorphous materials.”
The discovery establishes a clear structural principle: mechanically soft regions arise where disorder is embedded within medium-range order. This counterintuitive finding provides a practical guideline for developing amorphous solids that are both flexible and strong—benefiting applications from displays and coatings to energy devices.
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The article “Persistent homology elucidates hierarchical structures responsible for mechanical properties in covalent amorphous solids” will be published in Nature Communications at DOI: https://doi.org/10.1038/s41467-025-63424-z.
About The University of Osaka
The University of Osaka was founded in 1931 as one of the seven imperial universities of Japan and is now one of Japan's leading comprehensive universities with a broad disciplinary spectrum. This strength is coupled with a singular drive for innovation that extends throughout the scientific process, from fundamental research to the creation of applied technology with positive economic impacts. Its commitment to innovation has been recognized in Japan and around the world. Now, The University of Osaka is leveraging its role as a Designated National University Corporation selected by the Ministry of Education, Culture, Sports, Science and Technology to contribute to innovation for human welfare, sustainable development of society, and social transformation.
Website: https://resou.osaka-u.ac.jp/en
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[Press-News.org] Topology reveals the hidden rules of amorphous materials — Softness arises from hierarchical structures
For decades, the origins of “soft spots” in amorphous materials like glass remained a mystery. A new study shows that hierarchical atomic structures, uncovered through mathematical topology, are responsible for their mechanical behavior.
